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Low-temperature thermodynamic investigation of the sulphur organic salts (TMTTF)(2)PF6 and (TMTTF)(2)Br (TMTTF = tetramethyltetrathiafulvalene): II. Dynamical aspects (CROSBI ID 100555)

Prilog u časopisu | izvorni znanstveni rad | međunarodna recenzija

Lasjaunias, Jean-Claude ; Monceau, Pierre ; Starešinić, Damir ; Biljaković, Katica ; Carcel, C. ; Fabre, J.M. Low-temperature thermodynamic investigation of the sulphur organic salts (TMTTF)(2)PF6 and (TMTTF)(2)Br (TMTTF = tetramethyltetrathiafulvalene): II. Dynamical aspects // Journal of physics. Condensed matter, 14 (2002), 36; 8583-8594-x

Podaci o odgovornosti

Lasjaunias, Jean-Claude ; Monceau, Pierre ; Starešinić, Damir ; Biljaković, Katica ; Carcel, C. ; Fabre, J.M.

engleski

Low-temperature thermodynamic investigation of the sulphur organic salts (TMTTF)(2)PF6 and (TMTTF)(2)Br (TMTTF = tetramethyltetrathiafulvalene): II. Dynamical aspects

This contribution is in continuation of our preceding publication (Lasjaunias J C, Brison J P, Monceau P, Staresinic D, Biljakovic K, Carcel C and Fabre J M 2002 J. Phys.: Condens. Matter 14 837) in which we have considered general aspects of the low-temperature thermodynamical properties of the quasi-one-dimensional organic salts based on sulphur donors with different ground states: (TMTTF)(2)PF6 in the spin-Peierls state and (TMTTF)(2)Br (TMTTF = tetramethyltetrathiafulvalene) with commensurate spin modulation. In this part, part 11, we present our results on the dynamical aspects related to the non-equilibrium phenomena measured below I K. The metastable states excited to slightly higher temperature (by only a few per cent of the starting T-0) relax very slowly to the heat bath environment, depending on the duration of the heat pumping. We compare the features observed in the relaxation rates in these two sulphur compounds with those measured for the incommensurate spin-density-wave compound (TMTSF)(2)PF6. We discuss the possible nature of the long-living low-energy excitations lying at the origin of this complex dynamical behaviour, in relation to their ground states.

density-wave systems; phase-transitions; glass-transition; spin-glasses; specific heat; relaxations

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Podaci o izdanju

14 (36)

2002.

8583-8594-x

objavljeno

0953-8984

Povezanost rada

Fizika

Indeksiranost